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- Many early editions of Byron's works
- Letters and autograph materials of Catherine Gordon Byron, Thomas Moore, Edward Trelawny, Lady Byron, and others
- Books and material objects from the collection of Michael Rees, former Secretary of the International Council of Byron Societies
- Visual representations and portraits, such as Rembrandt Peale’s 1825 lithograph of Byron, as well as statuary, mezzotints and engravings, Staffordshire figuresbusts and Staffordshire figures, medals and plaques, drawings and engravings, and decorative and other material objects that demonstrate the impact of Byron’s life and works on his readers, both past and present
- Papers, correspondence, books and photographs from the collection of the late Leslie A. Marchand, author of Byron: A Biography and editor of Byron’s Letters and Journals.
- Byron-related papers of Jerome McGann, scholar of 18th century literature and culture, and editor of Byron: The Complete Poetical Works. This collection includes McGann's working files for the OET Byron edition, a large set of facsimiles of Byron MSS and associated Byroniana, and scholarly and critic materials used in his work on Byron and the historical period.
- The archives of the Byron Society of America
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